Detail projektu

THz Frequency Rapid Scan - Electron Spin Resonance spectroscopy for spin dynamics investigations of bulk and surface materials

Období řešení: 01.01.2018 — 31.12.2022

Zdroje financování

Evropská unie - Horizon 2020

- plně financující (2018-01-01 - 2022-01-01)

O projektu

Current high frequency electron spin resonance (HFESR) instruments suffer from the disadvantages of being limited to a single frequency and to tiny sample volumes. The study of spin dynamics at frequencies beyond a few hundred gigahertz is currently prohibitively difficult. These limitations are now preventing progress in dynamic nuclear polarization (DNP) and preclude the implementation of zero-field quantum computing. In order to revolutionize sensitivity in nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) by means of DNP techniques allowing to watch in real time molecular interactions or even to monitor how sophisticated systems (ribosomes) work, the HFESR methods have to be substantially improved. I will develop a novel and worldwide unique technique called broadband terahertz frequency rapid scan (FRaScan) ESR.

Klíčová slova
Electron Spin Resonance (ESR) spectroscopy, Spin dynamics, Dynamic Nuclear Polarization

Označení

714850

Originální jazyk

angličtina

Řešitelé

Útvary

Magneto-Optická a THz Spektroskopie
- příjemce (01.01.2018 - 01.01.2022)
Středoevropský technologický institut VUT
- odpovědné pracoviště (20.02.2017 - 27.08.2020)

Výsledky

SOJKA, A.; NEUGEBAUER, P. Terahertz Magnetic Resonance Spectrometer for Electron Spin Dynamics Investigations. Book of abstracts: V International School for Young Scientists on Magnetic Resonance and Magnetic Phenomena in Chemical and Biological Physics. Saint Petersburg: VVM Publishing Ltd., 2018. p. 229-229. ISBN: 978-5-9651-1175-6.
Detail

CALVO, R.; SARTORIS, R.; NASCIMENTO, O.; ŠEDIVÝ, M.; SOJKA, A.; NEUGEBAUER, P.; SANTANA, V. Quantum phase transitions probed by EPR spectra in dimeric spin arrays with supramolecular couplings. COORDINATION CHEMISTRY REVIEWS, 2023, vol. 480, no. 1, p. 1-25. ISSN: 1873-3840.
Detail

SOJKA, A.; MARTÍNEK, T.; ŠEDIVÝ, M.; ČALA, M.; SANTANA, V.; NEUGEBAUER, P. Development of a Terahertz Magnetic Resonance Spectrometer for Electron Spin Dynamics Investigations. 2018.
Detail

SOJKA, A.; ŠEDIVÝ, M.; SANTANA, V.; NEUGEBAUER, P. Terahertz Magnetic Resonance Spectrometer for Electron Spin Dynamics Investigations. 2018.
Detail

SOJKA, A.; ŠEDIVÝ, M.; MARTÍNEK, T.; MIDLÍKOVÁ, J.; ČALA, M.; SANTANA, V.; NEUGEBAUER, P. Terahertz Magnetic Resonance Spectrometer for Electron Spin Dynamics Investigations. Book of Abstracts CEITEC PhD & Postdoc Retreat. First edition. Žerotínovo nám. 617/9, 601 77 Brno, Czech Republic: Masaryk University, 2018. p. 54-54. ISBN: 978-80-210-8941-9.
Detail

Zdeg, I.; Al-Shami, A.; Tiouichi, G.; Absike, H.; Chaudhary, V.; Neugebauer, P.; Nouneh, K.; Belhboub, A.; Mounkachi, O.; El Fatimy, A. Electrical Transport Properties of Layered Black Phosphorus grown by Chemical Vapor Transport. Crystal Research and Technology, 2023, vol. 58, no. 1, ISSN: 1521-4079.
Detail

EL HAMMOUMI, M.; CHAUDHARY, V.; NEUGEBAUER, P.; EL FATIMY, A. Chemical vapor deposition: a potential tool for wafer scale growth of two-dimensional layered materials. Journal of Physics D - Applied Physics, 2022, vol. 55, no. 47, ISSN: 1361-6463.
Detail

ZHANG, X.; KAŠTYL, J.; CASAS LUNA, M.; HAVLÍČEK, L.; VONDRA, M.; BRUMMER, V.; SUKAČOVÁ, K.; MÁŠA, V.; TENG, S.; NEUGEBAUER, P. Microalgae-derived nanoporous biochar for ammonia removal in sustainable wastewater treatment. Journal of Environmental Chemical Engineering, 2022, vol. 10, no. 6, ISSN: 2213-3437.
Detail

SCHUBERT, M.; KNIGHT, S.; RICHTER, S.; KUEHNE, P.; STANISHEV, V.; RUDER, A.; STOKEY, M.; KORLACKI, R.; IRMSCHER, K.; NEUGEBAUER, P.; DARAKCHIEVA, V. Terahertz electron paramagnetic resonance generalized spectroscopic ellipsometry: The magnetic response of the nitrogen defect in 4H-SiC. Applied Physics Letters, 2022, vol. 120, no. 10, p. 1-6. ISSN: 0003-6951.
Detail

LAGUTA, O.; SOJKA, A.; MARKO, A.; NEUGEBAUER, P. Rapid scan ESR: A versatile tool for the spin relaxation studies at (sub)THz frequencies. Applied Physics Letters, 2022, vol. 120, no. 12, p. 1-7. ISSN: 0003-6951.
Detail

JURÁKOVÁ, J.; ŠALITROŠ, I. Co(II) single-ion magnets: synthesis, structure, and magnetic properties. Monatshefte für Chemie, 2022, vol. 153, no. 11, p. 1001-1036. ISSN: 1434-4475.
Detail

ŠEDIVÝ, M.; SOJKA, A.; LAGUTA, O. Progress in developement of software for FRaScan HFEPR spectrometer. 2 nd annual conference of the Magneto-Optical and THz Spectroscopy Research Group. Masłońskie, Polsko: 2019. p. 7-7.
Detail

LAGUTA, O.; TUČEK, M.; ŠEDIVÝ, M.; SOJKA, A.; SANTANA, V.; VAN SLAGEREN, J.; NEUGEBAUER, P. Multi-frequency rapid-scan HFEPR spectroscopy. Denver: Society for Applied Spectroscopy, 2019. p. 27-27.
Detail

ŠEDIVÝ, M.; SOJKA, A. Automated Alignment of a Quasi-Optical Table for a HFEPR Spectrometer. XIth EFEPR Conference, 1-5 September 2019, Bratislava, Book of Abstracts. Bratislava: SCHK, Slovak Chemistry Library, 2019. p. 133-133. ISBN: 978-80-8208-020-2.
Detail

St Marie, L.; El Fatimy, A.; Hruby, J.; Nemec, I.; Hunt, J.; Myers-Ward, R.; Gaskill, DK.; Kruskopf, M.; Yang, YF.; Elmquist, R.; Marx, R.; van Slageren, J.; Neugebauer, P.; Barbara, P. Nanostructured graphene for nanoscale electron paramagnetic resonance spectroscopy. Journal of Physics: Materials, 2020, vol. 3, no. 1, p. 14013-14021. ISSN: 2515-7639.
Detail

HRUBÝ, J.; DVOŘÁK, D.; SQUILLANTINI, L.; MANNINI, M.; VAN SLAGEREN, J.; HERCHEL, R.; NEMEC, I.; NEUGEBAUER, P. Co(II)-Based single-ion magnets with 1,1 '-ferrocenediyl-bis(diphenylphosphine) metalloligands. Dalton Transactions, 2020, vol. 49, no. 33, p. 11697-11707. ISSN: 1477-9234.
Detail

SOJKA, A.; ŠEDIVÝ, M.; LAGUTA, O.; MARKO, A.; SANTANA, V.; NEUGEBAUER, P. High-frequency EPR: current state and perspectives. In Electron Paramagnetic Resonance. Cambridge: The Royal Society of Chemistry, 2020. p. 214-252. ISBN: 978-1-83916-171-1.
Detail

ŠEDIVÝ, M.; SOJKA, A.; SANTANA, V.; GABRIŠ, A.; LAGUTA, O.; NEUGEBAUER, P. Software for versatile HFEPR spectrometer. EUROMAR : European Conference on Magnetic Resonance, 5th - 8th July, 2021, Ljubljana : book of abstracts. Ljubljana: Narodna in univerzitetna knjižnica, 2021. p. 270-270.
Detail

ZINKIEWITZ, M.; WOZNIAK, T.; KAZIMIERCZUK, T.; KAPUSCINSKI, P.; ORESZCZUK, K.; GRZESZCZYK, M.; BARTOŠ, M.; NOGAJEWSKI, K.; WATANABE, K.; TANIGUCHI, T.; FAUGERAS, C.; KOSSACKI, P.; POTEMSKI, M.; BABINSKI, A.; MOLAS, M. Excitonic Complexes in n-Doped WS2 Monolayer. NANO LETTERS, 2021, vol. 21, no. 6, p. 2519-2525. ISSN: 1530-6984.
Detail

MARKO, A.; SOJKA, A.; LAGUTA, O.; NEUGEBAUER, P. Simulation of nitrogen nuclear spin magnetization of liquid solved nitroxides. Physical Chemistry Chemical Physics, 2021, vol. 23, no. 32, p. 17310-17322. ISSN: 1463-9084.
Detail

BISWAS, S.; NEUGEBAUER, P. Lanthanide-Based Metal-Organic-Frameworks for Proton Conduction and Magnetic Properties. EUROPEAN JOURNAL OF INORGANIC CHEMISTRY, 2021, vol. 2021, no. 45, p. 4610-4618. ISSN: 1099-0682.
Detail

NAVARRO GIRALDO, J.; HRUBÝ, J.; VAVREČKOVÁ, Š.; SOJKA, A.; BARTOŠ, M.; NEMEC, I.; NEUGEBAUER, P.; HERCHEL, R.; MASARYK, L.; MONCOL, J. DFT study of Cobalt-based single-molecule magnet deposition on graphene. Manchester: 2021. p. 1 (1 s.).
Detail

NEMEC, I.; FELLNER, O.; INDRUCHOVÁ, B.; HERCHEL, R. Trigonally Distorted Hexacoordinate Co(II) Single-Ion Magnets. Materials, 2022, vol. 15, no. 3, p. 1064-1064. ISSN: 1996-1944.
Detail

SOJKA, A.; ŠEDIVÝ, M.; LAGIŇ, A.; GABRIŠ, A.; SANTANA, V.; LÁZNIČKA, T.; LAGUTA, O.; NEUGEBAUER, P. Sample Holders for Sub-THz Electron Spin Resonance Spectroscopy. IEEE TRANSACTIONS ON INSTRUMENTATION AND MEASUREMENT, 2022, vol. 71, no. 1, p. 1-12. ISSN: 1557-9662.
Detail

CHAUDHARY, V.; NEUGEBAUER, P.; MOUNKACHI, O.; LAHBABI, S.; EL FATIMY, A. Phosphorene-an emerging two-dimensional material: recent advances in synthesis, functionalization, and applications. 2D Materials, 2022, vol. 9, no. 3, p. 032001-1 (032001-23 p.)ISSN: 2053-1583.
Detail

ŠEDIVÝ, M.; HOFERKOVÁ, K.; SOJKA, A.: Very low temperature probe; Probe for electrical measurements in magnetic field and at cryogenic conditions. CEITEC BUT, Laboratory of EPR spectroscopy. URL: https://github.com/MatSevy/CEITEC-MOTES-VLTP. (funkční vzorek)
Detail

ŠEDIVÝ, M.; HRUBÝ, J.; LAGUTA, O.; SOLODOVNYK, A.; NEUGEBAUER, P.: bolometerSW; LTAUSA - V008 - Software pro charakterizaci grafénových bolometrů. MOTeS laboratory. (funkční vzorek)
Detail

SOLODOVNYK, A.; LAGUTA, O.; NEUGEBAUER, P.: OFF; LTAUSA19060 - V002 - Průchodka optických vláken pro THz FraScan spektrometr. MOTeS laboratory. (funkční vzorek)
Detail

SOLODOVNYK, A.; LAGUTA, O.; NEUGEBAUER, P.: ESH; LTAUSA19060 - V001 - EDMR držák vzorků pro THz FraScan spektrometr. MOTeS laboratory. (funkční vzorek)
Detail

SOJKA, A.; NEUGEBAUER, P.; LAGIŇ, A.: Chip Sample Holder; LTAUSA - V007 - Nerezonanční držák vzorků pro měření tenkých vrstev a testování nanometrových zařízení pomocí EPR spektrometru. MOTeS laboratory. (funkční vzorek)
Detail

HRUBÝ, J.; NEUGEBAUER, P.; SOJKA, A.; BARBARA, P.; ST. MARIE, L.: Fe4Ph on 9EM2 chip; LTAUSA19060 - V006 - Tvorba monovrsty JMM na grafenovém bolometru. MOTeS laboratory. (funkční vzorek)
Detail

ŠEDIVÝ, M.: Magnet module; Superconducing magnet module. CEITEC BUT, Magneto-Optical and THz Spectroscopy, laboratory of EPR spectroscopy.. URL: https://drive.google.com/open?id=1z5bJoKr2vwBhEJlF7RtBZVxb9Sezl52R. (software)
Detail

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