Activation cross section for the (n,2n) and (n,p) reactions on 103Rh, 48Ti and 52Cr from reaction threshold up to 25 MeV energy region

Activation cross section for the (n,2n) and (n,p) reactions on 103Rh, 48Ti and 52Cr from reaction threshold up to 25 MeV energy region

WoS Article

Activation and off-line γ-ray spectrometric methods were used to measure the ground and isomeric state (𝑛, 2𝑛) reaction cross section for 103Rh at two different neutron energies. The standard 27Al(𝑛, 𝛼)24Na reference reaction was used to normalise neutron flux. The proton beam from the 14UD BARC-TIFR Pelletron facility in Mumbai, India, was utilised to create high-energy quasi- monoenergetic neutrons via the 7Li(𝑝, 𝑛) reaction. Statistical model calculations including the level density, pre-equilibrium and optical potential model were performed using the TALYS (ver. 1.95) and EMPIRE (ver. 3.2.3) reaction codes. In addition, because of considerable discrepancies in measured data, the literature (𝑛, 𝑝) reaction cross section of 52Cr and 48Ti targets were examined theoretically in the present work. The measured cross sections are discussed and compared with the latest evaluated data of the FENDL-3.2b, CENDL-3.2, TENDL-2019, JENDL-5.0, and ENDF/B-VIII.0 libraries, and experimental data based on the EXFOR compilation. The theoretical investigation of the (𝑛, 2𝑛) reaction cross section was performed for the ground and isomeric state for the first time from reaction threshold to 25 MeV energies. The experimental data corresponding to the ground, isomeric state and isomeric ratio were reproduced consistently by the theoretical calculations. The present experimental results are good with certain literature data and theoretical values.

Activation and off-line γ-ray spectrometric methods were used to measure the ground and isomeric state (𝑛, 2𝑛) reaction cross section for 103Rh at two different neutron energies. The standard 27Al(𝑛, 𝛼)24Na reference reaction was used to normalise neutron flux. The proton beam from the 14UD BARC-TIFR Pelletron facility in Mumbai, India, was utilised to create high-energy quasi- monoenergetic neutrons via the 7Li(𝑝, 𝑛) reaction. Statistical model calculations including the level density, pre-equilibrium and optical potential model were performed using the TALYS (ver. 1.95) and EMPIRE (ver. 3.2.3) reaction codes. In addition, because of considerable discrepancies in measured data, the literature (𝑛, 𝑝) reaction cross section of 52Cr and 48Ti targets were examined theoretically in the present work. The measured cross sections are discussed and compared with the latest evaluated data of the FENDL-3.2b, CENDL-3.2, TENDL-2019, JENDL-5.0, and ENDF/B-VIII.0 libraries, and experimental data based on the EXFOR compilation. The theoretical investigation of the (𝑛, 2𝑛) reaction cross section was performed for the ground and isomeric state for the first time from reaction threshold to 25 MeV energies. The experimental data corresponding to the ground, isomeric state and isomeric ratio were reproduced consistently by the theoretical calculations. The present experimental results are good with certain literature data and theoretical values.

(n,2n) reaction; (n,p) reaction; cross sections; 7Li; neutron source; activation and off-line γ-ray spectrometric techniques; TALYS (ver. 1.95) code; EMPIRE (ver. 3.2.3) code

(n,2n) reaction; (n,p) reaction; cross sections; 7Li; neutron source; activation and off-line γ-ray spectrometric techniques; TALYS (ver. 1.95) code; EMPIRE (ver. 3.2.3) code

SINGH, R.; SINGH, N.; MEHTA, M.; CHAUHAN, R.; SURYANARAYANA, S.; MAKWANA, R.; NAYAK, B.; NAIK, H.; VARMUŽA, J.; KATOVSKÝ, K.

2024

27.07.2023

Elsevier B.V.

Radarweg 29 Millennium Tower Nizozemsko

1872-9800

Applied Radiation and Isotopes

200

October 2023

United States of America

1

13

13

https://www.sciencedirect.com/science/article/pii/S0969804323003020