Publication result detail

Bistable (Supra)molecular Switches on 3D-Printed Responsive Interfaces with Electrical Readout

MUÑOZ MARTIN, J.; REDONDO NEGRETE, E.; PUMERA, M.

Original Title

Bistable (Supra)molecular Switches on 3D-Printed Responsive Interfaces with Electrical Readout

English Title

Bistable (Supra)molecular Switches on 3D-Printed Responsive Interfaces with Electrical Readout

Type

WoS Article

Original Abstract

Molecular switching memories have gained great importance in recent years because of the current sharp increase in the production of consumer electronics. Herein, 3D-printed nanocomposite carbon electrodes (3D-nCEs) have been explored as unconventional responsive interfaces to electrically readout bistable molecular switches via electrochemical impedance spectroscopy as the output system. As a proof-of-concept, two different 3D-printed responsive interfaces have been devised using surface engineering for covalently anchoring (supra)molecular components that well-define two electrical states (on/off) driven by either electrical or optical stimuli. Accordingly, this work paves the way for the functionalization of 3D-nCEs through fundamental chemistry, opening up new horizons in unprecedented tailored 3D-printed responsive interfaces which could be utilized as potential (bio)sensors, (opto)electronic devices, or molecular logic gates.

English abstract

Molecular switching memories have gained great importance in recent years because of the current sharp increase in the production of consumer electronics. Herein, 3D-printed nanocomposite carbon electrodes (3D-nCEs) have been explored as unconventional responsive interfaces to electrically readout bistable molecular switches via electrochemical impedance spectroscopy as the output system. As a proof-of-concept, two different 3D-printed responsive interfaces have been devised using surface engineering for covalently anchoring (supra)molecular components that well-define two electrical states (on/off) driven by either electrical or optical stimuli. Accordingly, this work paves the way for the functionalization of 3D-nCEs through fundamental chemistry, opening up new horizons in unprecedented tailored 3D-printed responsive interfaces which could be utilized as potential (bio)sensors, (opto)electronic devices, or molecular logic gates.

Keywords

3D printing, 3D-printed electrodes, electrochemical impedance spectroscopy, graphene/PLA, supramolecular chemistry, optoelectronics, molecular logic gates

Key words in English

3D printing, 3D-printed electrodes, electrochemical impedance spectroscopy, graphene/PLA, supramolecular chemistry, optoelectronics, molecular logic gates

Authors

MUÑOZ MARTIN, J.; REDONDO NEGRETE, E.; PUMERA, M.

RIV year

2021

Released

11.12.2020

Publisher

ACS Publications

ISBN

1944-8252

Periodical

ACS Applied Materials & Interfaces

Volume

13

Number

11

State

United States of America

Pages from

12649

Pages to

12655

Pages count

7

URL

https://pubs.acs.org/doi/abs/10.1021/acsami.0c14487

BibTex

@article{BUT169905,
  author="Jose Maria {Muñoz Martin} and Edurne {Redondo Negrete} and Martin {Pumera}",
  title="Bistable (Supra)molecular Switches on 3D-Printed Responsive Interfaces with Electrical Readout",
  journal="ACS Applied Materials & Interfaces",
  year="2020",
  volume="13",
  number="11",
  pages="12649--12655",
  doi="10.1021/acsami.0c14487",
  issn="1944-8244",
  url="https://pubs.acs.org/doi/abs/10.1021/acsami.0c14487"
}