Publication detail

Surface Property Tuning of Methylammonium Lead Iodide by Plasma for Use in Planar Perovskite Solar Cells

SHEKARGOFTAR, M. POSPÍŠIL, J. DUGÁČEK, J. WEITER, M. HOMOLA, T.

Original Title

Surface Property Tuning of Methylammonium Lead Iodide by Plasma for Use in Planar Perovskite Solar Cells

Type

journal article in Web of Science

Language

English

Original Abstract

The demand for cheap and green energy as a replacement for fossil fuels has never been greater, and perovskite solar cells (PSCs) are among the leading means of meeting it. The surface properties of metal halide perovskite layers play crucial roles in the performance and durability of such cells. Consequently, a wide range of engineering processes for surface modification of perovskite layers has been investigated and among them is atmospheric pressure plasma (APP). Nevertheless, knowledge of the interaction between plasma and perovskite layers is still far from complete. In this work, CH3NH3PbI3 films were subjected to APP generated by a portable plasma source. A detailed understanding of band energy after plasma treatment is crucial to the investigation of the behavior of the perovskite layer. This study demonstrates a remarkable shift in the valence and conduction bands of a perovskite layer after plasma treatment, while band gap energy remains relatively constant. We found that short plasma treatment of perovskite layers resulted in higher performance and stability of PSCs.

Keywords

halide perovskite; atmospheric plasma; surface treatment; photoluminescence; energy band tuning

Authors

SHEKARGOFTAR, M.; POSPÍŠIL, J.; DUGÁČEK, J.; WEITER, M.; HOMOLA, T.

Released

28. 7. 2020

Publisher

AMER CHEMICAL SOC

Location

WASHINGTON

ISBN

2470-1343

Periodical

ACS OMEGA

Year of study

5

Number

29

State

United States of America

Pages from

18384

Pages to

18390

Pages count

7

URL

Full text in the Digital Library

BibTex

@article{BUT164814,
  author="Masoud {Shekargoftar} and Jan {Pospíšil} and Ján {Dugáček} and Martin {Weiter} and Tomáš {Homola}",
  title="Surface Property Tuning of Methylammonium Lead Iodide by Plasma for Use in Planar Perovskite Solar Cells",
  journal="ACS OMEGA",
  year="2020",
  volume="5",
  number="29",
  pages="18384--18390",
  doi="10.1021/acsomega.0c02179",
  issn="2470-1343",
  url="https://pubs.acs.org/doi/10.1021/acsomega.0c02179"
}